Accurate stacking engineering of MOF nanosheets as membranes for precise H₂ sieving.

2c , the pore size of monolayer nanosheet is exclusively influenced by the side chain size, while the obtained stacking aperture of each kind of MOF nanosheet stacks is co-influenced by the side chain size and the staggering degree, presenting a decreasing trend in stacking aperture with an increased sliding degree after the combination of the two factors.

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Both selectivity of H 2 /CH 4 and H 2 /CO 2 separation, as well as the H 2 permeance exhibit an increasing trend with the rise of H 2 concentration in the feed (Supplementary Fig. 28 ).

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