Adapting Atomic Configuration Steers Dynamic Half-Occupied State for Efficient CO<sub>2</sub> Electroreduction to CO.

39 In the cases of Fe, Co, and Cu ADTCs, one can find that as the applied potential was extended to larger cathodic values (−0.75 V RHE for Fe and Co and −0.95 V RHE for Cu), the overall CN values of all metal sites show a decreasing trend, which is below the four coordination.

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