Precise construction of Pd superstructures with modulated defect properties for solar-driven organic transformation.

1–5 Among various organic transformations, the oxidation of o -phenylenediamine (OPDA) to 2,3-diaminophenazine (DAP) is highly significant because DAP can serve as a pivotal intermediate in manufacturing with broad utility in various fields ( e.g. , production of conductive polymers, synthesis of carbon dots, detection of peroxides in analytical chemistry, and immunoassays). 6,7 Since OPDA is carcinogenic and toxic, the oxidation of OPDA may cause the degradation of organic pollutants.

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