Tautomer aspects in the excited-state dynamics in 2-thiocytosine: intersystem crossing in the absence of the thiocarbonyl group.

The lifetime τ 1 , which captures both the motion out of the FC region to the S π 1 minima and the depopulation of S π 1 , shows a decreasing trend with increasing vibrational excitation, i.e. , toward shorter pump wavelengths.

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