This research represents a curiosity-driven exploration that yielded highly significant observations regarding the ability of the metal–organic multitopic acceptor to simultaneously engage in halogen bonding with a large number of halogen bond donors (up to five) due to the presence of an acceptor species, the isothiocyanate sulfur atom, which forms a robust I⋯SCN synthon.
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Higher-order metal-organic halogen-bonded cocrystals relying on a single supramolecular synthon.
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