Solubility, speciation and local environment of chlorine in zirconolite glass-ceramics for the immobilisation of plutonium residues.

15% of total, is consistent with dominant Ln–O co-ordination in chloride bearing aluminosilicate glasses, in agreement with Ponader and Brown and is expected to be at the margin of significance in analysis of Ln L 3 EXAFS data acquired from such disordered materials.

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