Large Hyperfine Coupling Arising from Pseudo-<sup>2</sup>S Ground States in a Series of Lutetium(II) Metallocene Complexes.

Across the three Lu 2+ metallocene complexes, varying degrees of axiality act to further fine-tune the core magnetic properties and establish a clear trend among the geometric structure, crystal field axiality, and s-orbital parentage of the singly occupied molecular orbitals.

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