Modulating CO<sub>2</sub> electroreduction pathways through controlled ionomer arrangement on catalyst surfaces via solvent dispersion.

The resulting CO 2 RR performance reveals a clear trend: Cu-NR electrodes prepared in low-ε solvents favor both C–C coupling and the HER, with the additional capability of CH 4 production, while those prepared in high-ε solvents predominantly favor CO formation.

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